Mr. Larrain spent his early career as a painter, and he came to view his ultimate medium, photography, as painting with light. Over the course of his career, he shot for magazines including Rolling Stone, Esquire, Vogue and Time, and he created shimmering, at times dreamlike, portraits of John Lennon and Yoko Ono, Mikhail Baryshnikov, Laurie Anderson, Norman Mailer and many others.